Volume 37 Issue 4
Dec.  2023
Turn off MathJax
Article Contents
WEI Shiping, LI Cong. Design and optimization of dimethyl ether reforming reactor for hydrogen production[J]. Journal of Shanghai University of Engineering Science, 2023, 37(4): 335-342. doi: 10.12299/jsues.22-0242
Citation: WEI Shiping, LI Cong. Design and optimization of dimethyl ether reforming reactor for hydrogen production[J]. Journal of Shanghai University of Engineering Science, 2023, 37(4): 335-342. doi: 10.12299/jsues.22-0242

Design and optimization of dimethyl ether reforming reactor for hydrogen production

doi: 10.12299/jsues.22-0242
  • Received Date: 2022-08-09
  • Publish Date: 2023-12-30
  • A frustum of a cone for dimethyl ether (DME) steam reforming hydrogen production was designed, and the numerical model of DME steam reforming hydrogen production reaction system was established. The numerical model was solved by COMSOL software, the numerical results of simulation and experiment were basically consistent. By optimizing the structure of the reforming reactor, higher DME conversion rate was obtained. The influence of the cone change on the reforming reaction , and the influence of reaction conditions on DME conversion and hydrogen production were analyzed. The results showed that higher hydrogen yield and thermal efficiency can be obtained When increasing the taper within a certain range. Through structural optimization, the DME steam reforming reaction system can obtain 92.21% DME conversion and 90.54% hydrogen production rate. The highest thermal efficiency is 74.6%.
  • loading
  • [1]
    ADENIYI A G, IGHALO J O, ELETTA O A A. Process integration and feedstock optimisation of a two-step biodiesel production process from jatropha curcas using aspen plus[J] . Chemical Product and Process Modeling,2018,14(2):2018 − 0055.
    [2]
    FAN F Y, ZHAO L, HOU H, ZHANG Q. Insights into the CO formation mechanism during steam reforming of dimethyl ether over NiO/Cu-based catalyst[J] . Industrial & Engineering Chemistry Research,2019,58(8):3440 − 3449.
    [3]
    刘江华. 氢能源: 未来的绿色能源[J] . 现代化工,2006(S2):10 − 13,15. doi: 10.16606/j.cnki.issn0253-4320.2006.s2.003
    [4]
    KAJORNSAK F, NAWIN V, WIWUT T. Evaluation of the thermodynamic equilibrium of the autothermal reforming of dimethyl ether[J] . International Journal of Hydrogen Energy,2011,36(10):5865 − 5874. doi: 10.1016/j.ijhydene.2011.02.027
    [5]
    SONG J W, CHOI M Y, LEE J, et al. Improvement of fuel economy and greenhouse gases reduction in gasoline powered vehicles through the TWC-NOx trap catalyst[J] . International Journal of Automotive Technology,2020,21(2):441 − 449. doi: 10.1007/s12239-020-0041-8
    [6]
    SWMWISBERGER T A, BORUP R L. Thermodynamic equilibrium calculations of dimethyl ether steam reforming and dimethyl ether hydrolysis[J] . Journal of Power Soures,2005,152(10):87 − 96.
    [7]
    FENG D M, WANG Y Y, WANG D, et al. Steam reforming of dimethyl ether over Cu-ZnO-Al2O3-ZrO2 + ZSM-5: A kinetic study[J] . Chemical Engineering Journal,2009,146(2):477 − 485.
    [8]
    WANG S, ISHIHARA T, TAKITA Y. Partial oxidation of dimethyl ether over various supported metal catalysts[J] . Applied Catalysis A: General,2002,228(1/2):167 − 176. doi: 10.1016/S0926-860X(01)00985-1
    [9]
    LI C, GAO Y, WU C. Modeling and simulation of hydrogen production from dimethyl ether steam reforming using exhaust gas[J] . International Journal of Energy Research,2015,39(9):1272 − 1279. doi: 10.1002/er.3330
    [10]
    寇素原, 王晓蕾, 任克威, 等. 二甲醚水蒸气重整制氢过程的热力学分析[J] . 天然气化工(C1化学与化工),2009,34(1):35 − 40.
    [11]
    CHEN Y, ZHANG C, WU R, et al. Methanol steam reforming in microreactor with constructal tree-shaped network[J] . Journal of Power Sources,2011,196(15):6366 − 6373. doi: 10.1016/j.jpowsour.2011.03.044
    [12]
    YAO F, CHEN Y, PETERSON G P. Hydrogen production by methanol steam reforming in a disc microreactor with tree-shaped flow architectures[J] . International Journal of Heat and Mass Transfer,2013,64:418 − 425. doi: 10.1016/j.ijheatmasstransfer.2013.04.057
    [13]
    AN H, LI A, SASMITO A P, et al. Computational fluid dynamics (CFD) analysis of micro-reactor performance: Effect of various configurations[J] . Chemical Engineering Science,2012,75:85 − 95. doi: 10.1016/j.ces.2012.03.004
    [14]
    CHEN S Y, Li C, REN H J. Design and optimization of reforming hydrogen production reaction system for automobile fuel cell[J] . International Journal of Hydrogen Energy,2021,46(49):25252 − 25263. doi: 10.1016/j.ijhydene.2021.05.035
    [15]
    XU D, LI C. Design and optimization of dimethyl ether steam-reforming reactor[J] . Journal of Energy Engineering,2022,148(2):1943.
    [16]
    ZHANG T Q, OU K, JUNG S H, et al. Dynamic analysis of a PEM fuel cell hybrid system with an on-board dimethyl ether (DME) steam reformer (SR)[J] . International Journal of Hydrogen Energy,2018,43(29):13521 − 13531. doi: 10.1016/j.ijhydene.2018.05.098
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Figures(11)  / Tables(1)

    Article Metrics

    Article views (194) PDF downloads(136) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return